3B2v7:51c                                                                                       ED:Chanakshi
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                                             Journal of Magnetism and Magnetic Materials ] (]]]]) ]]]­]]]
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7              Micromagnetic structures in square magnetic nanodots
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      M. Maicasa, M.A. Riveroa, E. L!opeza,*, M.C. S!ancheza, C. Arocab, P. S!anchezb
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                       a Departmento de F!isica de Materiales, Facultad de CC. F!isicas, Univ. Complutense, 28040 Madrid, Spain
                                        b
13                                           I.S.O.M., E.T.S.I. Telecomunicaci!on, Univ. Polit!ecnica, 28040 Madrid, Spain

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      Abstract
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         The structure of magnetization in magnetic square dots is studied in the range of tens of nanometer by means of
19    micromagnetic simulations. Two magnetic configurations are found, diagonal and vortex structures for thin films, flower
      and vortex for magnetic nanocubes and a hybrid flower in bulk and vortex near the surfaces for dots with thicknesses
21    larger than dot edge length. r 2002 Published by Elsevier Science B.V.

23    Keywords: Micromagnetism; Nanodot; Magnetostatic; Simulation

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         The rapidly decreasing size of magnetic devices has                             100 erg=cm3 parallel to the x-axis has also been
27    increased the interest in magnetic structures for particles                        considered. The criterion for convergence used was a            57
      at nanoscale dimensions. Nanoimprint lithography can                               maximum variation in magnetization director cosines
29    result in magnetic nanostructures which seem applicable                            smaller than 2   10 4 and the grid cells used were cubes        59
      for ultrahigh recording media [1]. For such high                                   of 3:125 nm edge length. These latter parameters were
31    densities perpendicular recording seems to be appro-                               used in all calculations in order to keep the same error        61
      priate [2]. Magnetic dots with a thickness higher than                             when making comparisons.
33    dot base dimensions exhibit perpendicular magnetic                                   While anisotropy can play an important role in                63
      orientation. This makes an interesting review of the                               magnetic distribution in dots with dimensions in the
35    magnetic layer thickness influence on magnetic struc-                              range of hundreds of nanometers [5] at the scale of tens        65
      tures for magnetic dots.                                                           of nanometers, magnetization distribution appears
37       Micromagnetic simulations prove to be specially                                 mainly dependent on exchange and magnetostatic                  67
      appropriate for nanoparticles. Calculations with cell                              interactions. From the exchange point of view, magne-
39    dimensions over the exchange length may result in                                  tization tries to get nearly parallel in order to reduce the    69
      computational errors due to an undervaluated exchange                              exchange contribution. From the magnetostatic point of
41    energy. On the other hand, magnetostatic energy                                    view, magnetization tries to avoid surface poles. The           71
      evaluation becomes very time consuming for grids with                              smaller the sample is, the more important the exchange
43    a large number of cells. At nanoscale dimensions we can                            becomes and so dots of few tens of nanometers exhibit           73
      work with grids with not a large number of cells, keeping                          nearly parallel magnetic configurations. For bigger dots
45    cell dimensions below the exchange length. Calculations                            magnetization tries to avoid surface poles and dots             75
      have been performed following a Labonte scheme [3]                                 exhibit circular rotating magnetization configurations.
47    minimizing exchange, anisotropy and magnetostatic                                  Certain transition dimensions appear for which these            77
      energies. The evaluation of magnetostatic energy is                                two different structures have nearly the same energy.
49    accelerated                                                                                                                                        79

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        *Correspo         UNCORRECTED PROOF
                       by means of the fast Fourier transform                              For thin film magnetic dots calculations lead to two
      technique [4]. Parameters used in the calculations are                             different configurations as shown in Fig. 1 [6,7], one
      typical for permalloy Ms ź 800 emu=cm3; Aex ź 1:3                                  with magnetization parallel to the square diagonal,
      10 6 erg=cm and an uniaxial anisotropy of K ź                                      diagonal, and another with rotating magnetization,
                                                                                         vortex. A third structure can be reached with magnetiza-        83
                     nding author. Tel.: +34-91-3944549; fax: +34-91-                    tion parallel to dot edge although with higher energy
55    3944547.                                                                           than that with magnetization parallel to the dot                85
          E-mail address: elolopez@eucmax.sim.ucm.es (E. L!opez).

      0304-8853/01/$ - see front matter r 2002 Published by Elsevier Science B.V.
      PII: S 0 3 0 4 - 8 8 5 3 ( 0 1 ) 0 1 3 5 7 - 9



                                                            MAGMA : 8775
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      2                        M. Maicas et al. / Journal of Magnetism and Magnetic Materials ] (]]]]) ]]]­]]]

1                                                                        Table 2                                                              49
                                                                         Magnetic energy in 50   50 nm dots for different thicknesses
3                                                                                                                                             51
                                                                         Thickness (nm)            Diagonal (erg)           Vortex (erg)

5                                                                        6                         6:6   10 12              No convergence    53
                                                                         12                        2:0   10 11              2:7   10 11
7                                                                        25                        5:8   10 11              5:2   10 11       55
                                                                         50                        9:9   10 11              9:9   10 11
9                                                                        100                       No convergence           1:7   10 10       57

11                                                                                                                                            59
      Fig. 1. (a) diagonal and (b) vortex magnetization configura-
13    tions in a 50   50 nm base, 12:5 nm height magnetic dot.                                                                                61

15                                                                                                                                            63
      Table 1
17    Magnetic energy in a 10 nm thick dot for different dot                                                                                  65
      dimensions
19                                                                                                                                            67
      Dot edge (nm)          Diagonal (erg)        Vortex (erg)

21    25                     5:6   10 12           No convergence         (a)                                (b)                              69
      50                     1:4   10 11           2:1   10 11
23    100                    3:3   10 11           3:0   10 11                                                                                71
      200                    6:9   10 11           4:3   10 11

25                                                                                                                                            73

27    diagonal. Table 1 shows the magnetic energy for                                                                                         75
      different dot dimensions. The smaller the dot, the more
29    stable is the diagonal state, while the bigger the sample                                                                               77
      the more stable is the vortex state.                                (c)
31          The effect of the thickness on the magnetic energy                                                                                79
                                                                         Fig. 2. Magnetization in (a) bottom, (b) middle and (c) top
      figures can be seen in Table 2. The diagonal state                 layers in a 50   50 nm base, 100 nm height magnetic dot.
33    becomes more stable for thinner sample. No conver-                                                                                      81
      gence is even reached for the vortex state for very small
35    thicknesses. For the cube, the diagonal state dissapears                                                                                83
      in favor of the flower state [8]. It can be seen that the          References
37    energy of the flower and vortex states are very similar for                                                                             85
      a nanocube of 50 nm edge length. For a thicker sample a            [1] L. Torres, et al., J. Appl. Phys. 85 (8) (1999) 6208.
39    new magnetic distribution appears as a mix of the flower           [2] L. Abelmann, et al., J. Appl. Phys. 87 (9) (2000) 5538.          87
      and vortex structures. Fig. 2 shows the magnetic layout            [3] A.E. LaBonte, J. Appl. Phys. 40 (1969) 2450.
41    in the lower, middle and upper layers in a 50   50 nm2             [4] M. Mansuripur, R. Giles, IEEE Trans. Magn. 24 (1988)             89
      base, 100 nm height magnetic dot. In this case the                         2326.
43    magnetization in the center is parallel to the large axis          [5] R.P. Cowburn, J. Phys. D: Appl. Phys. 33 (2000) R1­R16.          91
      while upper and lower layers exhibit a vortex-like                 [6] J. Miltat, et al., Proceedings of the Congress on Trends in
45    structure with the same distribution but opposite                          nanotechnology, Toledo, Spain, 2000.                         93
      directions.                                                        [7] M.A. Rivero, et al., Proceedings of the Congress on Trends
47          This work was partially supported by CICYT projects                  in nanotechnology, Toledo, Spain, 2000.
                                                                         [8] M.E. Schabes, H.N. Bertram, J. Appl. Phys. 64 (3) (1988)         95
      MAT98-0824-C02 and MAT2000-0330-P4-03.                                     1347.
                       UNCORRECTED PROOF