FN ISI Export Format VR 1.0 PT J AU Haas, M Realo, E Winkler, H Meyer-Klaucke, W Trautwein, AX TI SYNFOS SO HYPERFINE INTERACTIONS NR 10 AB An expression for the amplitude of a pulse of synchrotron radiation coherently scattered in the forward direction by a Mossbauer absorber consisting of randomly oriented paramagnetic iron-containing molecules (for example, a frozen solution of a Fe-57 protein) in an applied magnetic field is derived from the theory of gamma optics. It is assumed that the hyperfine splittings present in the Mossbauer nuclei can be described in the framework of the spin-Hamiltonian formalism. In the general case of a thick Mossbauer sample of this kind the response on an incident monochromatic and fully polarized beam cannot be given analytically because of the integrations involved. How nuclear forward-scattering for this general case is evaluated in the program package called SYNFOS is outlined. CR ABRAGAM A, 1951, P ROY SOC LOND A MAT, V205, P135 AFANASEV AM, 1965, ZH EKSP TEOR FIZ, V48, P327 BLUME M, 1968, PHYS REV, V171, P417 EDMONDS RA, 1957, ANGULAR MOMENTUM QUA HAAS M, 1997, PHYS REV B, V56, P14082 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1968, PHYS REV, V169, P315 KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 KNESE K, 1995, THESIS U LEIPZIG TRAUTWEIN AX, 1991, STRUCT BOND, V78, P1 TC 0 BP 189 EP 195 PG 7 JI Hyperfine Interact. PY 2000 VL 125 IS 1-4 GA 288VZ J9 HYPERFINE INTERACTIONS UT ISI:000085586300010 ER PT J AU Spiering, H Deak, L Bottyan, L TI EFFINO SO HYPERFINE INTERACTIONS NR 20 AB The program EFFINO (Environment For FItting Nuclear Optics) evaluates Mossbauer absorption and time spectra both in nuclear forward scattering and in grazing incidence reflection geometry. Time-integral prompt and delayed angular scan spectra are also treated. The time spectra are calculated by Fourier transformation from frequency to time domain. The electric quadrupole and magnetic dipole fields at the nuclear sites are considered static at present. The specimen in both forward scattering and grazing incidence is assumed to be a multilayer, with individual thickness and interface roughness (the latter only for the grazing incidence case at present) and electronic index of refraction. Up to eight different layers plus eight repetition periods of those layers are treated. Each layer may contain zero to eight nuclear sites (zero in all layers being prompt X-ray reflectivity), with their own effective thickness or (for grazing incidence) their own complex nuclear index of refraction. From the forward scattering amplitude, a differential 4 x 4 propagation matrix is constructed for each layer. Several experimental spectra of the same or different type(s) can be fitted simultaneously. Correlations between parameters of the same or of different spectra can be introduced. CR *J GUT U, 1982, AN CHEM AN CHEM AFANASEV AM, 1965, ZH EKSP TEOR FIZ, V21, P215 ANDREEVA MA, 1994, SOV PHYS JETP, V78, P965 ANDREEVA MA, 1986, VESTN MOSK U FIZ AS+, V27, P57 BLUME M, 1968, PHYS REV, V171, P417 BORZDOV GN, 1976, ZH PRIKL SPEKTROSK, V25, P526 DEAK L, 1999, CONDENSED MATTER STU DEAK L, IN PRESS COMMON ANIS DEAK L, 1996, PHYS REV B, V53, P6158 FEDOROV FI, 1976, TEORIA GIROTROPII GRANT RW, 1968, PHYS REV, V171, P417 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1968, PHYS REV, V169, P315 HANNON JP, 1984, PHYS REV B, V32, P5068 IRKAEV SM, 1993, NUCL INSTRUM METH B, V74, P545 IRKAEV SM, 1993, NUCL INSTRUM METH B, V74, P554 KULCSAR K, 1971, P INT C MOSSB SPECTR, P594 MULLER EW, 1982, MOSFUN LAB REPORT AN ROHLSBERGER R, 1994, THESIS U HAMBURG SPIERING H, 1978, HYP INTERACT, V120, P265 TC 1 BP 197 EP 204 PG 8 JI Hyperfine Interact. PY 2000 VL 125 IS 1-4 GA 288VZ J9 HYPERFINE INTERACTIONS UT ISI:000085586300011 ER PT J AU Smirnov, GV TI General properties of nuclear resonant scattering SO HYPERFINE INTERACTIONS NR 47 AB The process of nuclear resonant scattering resonant scattering is considered on the basis of an optical model. The coherent properties coherent properties of the radiation and scattering mechanism are described. The complementary pictures of gamma- ray resonant scattering in energy and time domains are presented. Special attention is paid to scattering of a gamma quantum by an ensemble of nuclei. The central concept of the theory of nuclear resonant scattering, the nuclear exciton, nuclear exciton as a delocalized nuclear excitation, is described in detail. It is shown that both temporal and spatial aspects of coherence play a crucial role in the evolution of the nuclear exciton. A large place is given to the analysis of resonant scattering of synchrotron radiation by nuclear ensembles. 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PY 1999 VL 123 IS 1-8 GA 288VG J9 HYPERFINE INTERACTIONS UT ISI:000085584700004 ER PT J AU Hannon, JP Trammell, GT TI Coherent gamma-ray optics SO HYPERFINE INTERACTIONS NR 129 AB With the advent of high brightness synchrotron radiation sources, an important new field has been opened up involving coherent nuclear excitations induced by synchrotron radiation pulses traversing a piece of matter. We review the theory of coherent resonant gamma-ray optics, including some of the interesting new phenomena which occur when systems of nuclei are excited by synchrotron radiation pulses, such as the creation of nuclear exciton states, superradiant and subradiant decay, spatially coherent quantum beats, and temporal Pendellosung. We also discuss the relation between the nuclear exciton states and multi-photon Dicke superradiance and gamma- ray lasers, and comment on neutron phasors and neutron superradiance in resonant neutron optics. The interesting features of coherent enhancement, superradiant decay, and dynamical beats are discussed from the fundamental perspective of the radiative normal modes of a system of nuclear resonators. 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1968, ZH EKSP TEOR FIZ, V27, P819 KIKUTA S, 1994, RESONANT ANOMALOUS X, P635 KOHN VG, 1994, SOV PHYS JETP, V78, P357 LAMB WE, 1964, PHYS REV, V134, PA1429 LANDAU LD, 1960, ELECTRODYNAMICS CONT, P288 LLOYD SP, 1951, PHYS REV, V83, P716 LOVESEY SW, 1984, THEORY NEUTRON SCATT LU F, 1989, THESIS RICE U LUO J, 1993, PHYS REV LETT, V71, P287 LUO J, 1994, THESIS RICE U MIRZABABAEV RM, 1971, PHYS LETT A, V37, P441 MOSSBAUER RL, 1975, ANOMALOUS SCATTERING, P463 MUZIKARZH C, 1962, SOV PHYS JETP, V14, P833 PARAK F, 1971, Z PHYS, V244, P456 PATTERSON AL, 1934, PHYS REV, V46, P372 PODGORETSKI MI, 1961, SOV PHYS JETP, V12, P1023 ROSE ME, 1957, ELEMENTARY THEORY AN, P32 RUBY SL, 1974, J PHYS PARIS C, V6, P209 SAKURAI JJ, 1973, ADV QUANTUM MECH, P56 SCHAWLOW AL, 1958, PHYS REV, V112, P1940 SHEN TX, 1991, THESIS RICE U SHVYDKO YV, 1998, PHYS REV B, V57, P3552 SMIRNOV GV, 1969, JETP LETT, V9, P123 SMIRNOV GV, 1994, RESONANT ANOMALOUS X, P609 STURHAHN W, 1995, PHYS REV LETT, V74, P3832 SZOKE A, 1986, AIP 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P355 VONLAUE M, 1960, ROENTGENSTRAHL INTER, P430 WENDIN G, 1980, PHYS SCRIPTA, V21, P535 WINKLER H, 1983, Z PHYS B CON MAT, V49, P331 WORD RE, 1981, PHYS REV B, V24, P2430 ZARETSKII DF, 1965, SOV PHYS JETP, V21, P243 TC 0 BP 127 EP 274 PG 148 JI Hyperfine Interact. PY 1999 VL 123 IS 1-8 GA 288VG J9 HYPERFINE INTERACTIONS UT ISI:000085584700006 ER PT J AU Shvyd'ko, YV TI Coherent nuclear resonant scattering of X-rays: Time and space picture SO HYPERFINE INTERACTIONS NR 56 AB The problem of coherent resonant scattering of X-rays by an ensemble of nuclei is solved directly in time and space. In a first step the problem with a single coherently scattered beam is considered - nuclear forward scattering. The wave equation describing the propagation of the radiation through the nuclear ensemble is derived. It is a first order integro-differential equation. Its kernel is a double time function K(t, (t) over tilde) which represents the coherent single scattering response of the nuclear system at time t to excitation at (t) over tilde. The kernel is defined by the character of the interactions the nuclei experience with the environment and by the character of their motion. A general procedure of solution of the wave equation is introduced which is independent of the type of kernel. In a second step the wave equation is generalized to the case of many coherently scattered beams, which is, e.g., the case of nuclear Bragg diffraction. Kernels of the wave equations are derived for some particular cases: collective motion of nuclei in space, thermal lattice vibrations, time-independent hyperfine interactions, and time- dependent hyperfine interactions due to external magnetic-field switching. CR AFANASEV AM, 1963, SOV PHYS JETP, V18, P1139 AFANASEV AM, 1965, ZH EKSP TEOR FIZ, V21, P215 AKHIEZER AI, 1965, QUANTUM ELECTRODYNAM ALEKSANDROV PA, 1975, SOV PHYS JETP, V40, P360 ALLEN L, 1975, OPTICAL RESONANCE 2 BERESTETSKII VB, 1971, RELATIVISTIC QUANTUM BLUM K, 1981, DENSITY MATRIX THEOR BLUME M, 1968, PHYS REV, V171, P417 BLUME M, 1967, PHYS REV, V165, P446 BURNHAM DC, 1969, PHYS REV, V188, P667 DEAK L, 1996, PHYS REV B, V53, P6158 GERDAU E, 1986, PHYS REV LETT, V57, P1141 HAAS M, 1997, PHYS REV B, V56, P14082 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1968, PHYS REV, V169, P315 HANNON JP, 1985, PHYS REV B, V32, P5068 HANNON JP, 1985, PHYS REV B, V32, P6363 HASTINGS JB, 1991, PHYS REV LETT, V66, P770 KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 KAGAN Y, 1973, Z NATURFORSCH A, VA 28, P1351 KAGAN Y, 1968, ZH EKSP TEOR FIZ, V27, P819 KIKUTA S, 1994, HYPERFINE INTERACT, V90, P335 KOHN VG, 1995, J PHYS-CONDENS MAT, V7, P7589 KOHN VG, 1998, PHYS REV B, V57, P5788 LANDAU LD, 1970, QUANTUM MECH NON REL LAUBEREAU A, 1978, REV MOD PHYS, V50, P607 LYNCH FJ, 1960, PHYS REV, V120, P513 MARADUBIN AA, 1971, THEORY LATTICE DYNAM MESSIAH A, 1962, QUANTUM MECH, V2 MITSUI T, 1997, JPN J APPL PHYS 1, V36, P6525 ROHLSBERGER R, 1997, HASYLAB, P933 ROHLSBERGER R, UNPUB PHYS REV LETT SHVYDKO YV, 1994, EUROPHYS LETT, V26, P215 SHVYDKO YV, 1993, EUROPHYS LETT, V22, P305 SHVYDKO YV, HE181 ESRF SHVYDKO YV, 1994, HYPERFINE INTERACT, V90, P287 SHVYDKO YV, 1993, J PHYS-CONDENS MAT, V5, P1557 SHVYDKO YV, 1992, J PHYS-CONDENS MAT, V4, P2663 SHVYDKO YV, 1991, JETP LETT+, V53, P69 SHVYDKO YV, 1991, JETP LETT+, V53, P231 SHVYDKO YV, 1999, PHYS REV B, V59, P9132 SHVYDKO YV, 1998, PHYS REV B, V57, P3552 SHVYDKO YV, 1996, PHYS REV B, V54, P14942 SHVYDKO YV, 1995, PHYS REV B, V52, PR711 SHVYDKO YV, 1996, PHYS REV LETT, V77, P3232 SINGWI KS, 1960, PHYS REV, V120, P1093 SMIRNOV GV, 1997, AIP CONF PROC, P323 SMIRNOV GV, 1996, HYPERFINE INTERACT, V97-8, P551 SMIRNOV GV, 1995, PHYS REV B, V52, P3356 SMIRNOV GV, 1996, PHYS REV LETT, V77, P183 STURHAHN W, 1994, PHYS REV B, V49, P9285 TAKAGI S, 1962, ACTA CRYSTALLOGR, V15, P1311 TRAMMELL GT, 1962, PHYS REV, V126, P1045 TRAMMELL GT, 1978, PHYS REV B, V18, P165 VANBURCK U, 1992, PHYS REV B, V46, P6207 VANHOVE L, 1955, PHYS REV, V55, P190 TC 0 BP 275 EP 299 PG 25 JI Hyperfine Interact. PY 1999 VL 123 IS 1-8 GA 288VG J9 HYPERFINE INTERACTIONS UT ISI:000085584700007 ER PT J AU Rohlsberger, R TI Theory of X-ray grazing incidence reflection in the presence of nuclear resonance excitation SO HYPERFINE INTERACTIONS NR 37 AB The dynamical theory of nuclear resonant diffraction is applied to the case of grazing incidence reflection. The solution of the dynamical equations is obtained by evaluation of a matrix exponential. This formalism is applied to grazing incidence reflection from arbitrary stratified media. However, the basic formalism is not restricted to this case, but can be used to describe a wide range of diffraction phenomena. This is demonstrated in the case of grazing incidence diffraction from gratings in the n-beam case. Moreover, the theory is extended to describe the influence of surface and boundary roughness. CR AZZAM RMA, 1987, ELLIPSOMETRY POLARIZ BADER S, 1994, ULTRATHIN MAGNETIC S, V2, P297 BANSMANN J, IN PRESS BATTERMAN BW, 1964, REV MOD PHYS, V36, P681 BLAND JAC, 1994, ULTRATHIN MAGNETIC S, V1, P305 BLUME M, 1985, J APPL PHYS, V57, P3615 BLUME M, 1968, PHYS REV, V171, P417 BORN M, 1978, PRINCIPLES OPTICS BOTTYAN L, 1998, HYPERFINE INTERACT, V113, P295 DEAK L, 1996, PHYS REV B, V53, P6158 DEBOER DKG, 1991, PHYS REV B, V44, P498 FENG YP, 1993, PHYS REV LETT, V71, P537 GROTE M, 1991, EUROPHYS LETT, V17, P707 HANNON JP, 1968, PHYS REV, V169, P315 HANNON JP, 1985, PHYS REV B, V32, P5068 HANNON JP, 1985, PHYS REV B, V32, P6363 HANNON JP, 1988, PHYS REV LETT, V61, P1245 HANNON JP, 1979, PHYS REV LETT, V43, P636 KROL A, 1988, PHYS REV B, V38, P8579 LAGOMARSINO S, 1996, J APPL PHYS, V79, P4471 LUCAS CA, 1991, EUROPHYS LETT, V14, P343 LUO J, 1993, PHYS REV LETT, V71, P287 NEVOT L, 1980, REV PHYS APPL, V15, P761 NIESEN L, 1998, PHYS REV B, V58, P8590 ROHLSBERGER R, 1994, 9404 DESY HASYLAB ROHLSBERGER R, 1992, EUROPHYS LETT, V18, P561 ROHLSBERGER R, 1994, HYPERFINE INTERACT, V92, P1107 ROHLSBERGER R, 1997, NUCL INSTRUM METH A, V394, P251 ROHLSBERGER R, 1993, Z PHYS B CON MAT, V92, P489 SIDDONS DP, 1995, NUCL INSTRUM METH B, V103, P371 SIDDONS DP, 1990, PHYS REV LETT, V64, P1967 SINHA SK, COMMUNICATION STURHAHN W, 1994, PHYS REV B, V49, P9285 TOELLNER TS, 1995, APPL PHYS LETT, V67, P1993 TOLAN M, 1992, EUROPHYS LETT, V20, P223 VIDAL B, 1984, APPL OPTICS, V23, P1794 WANG J, 1992, SCIENCE, V258, P775 TC 0 BP 301 EP 325 PG 25 JI Hyperfine Interact. PY 1999 VL 123 IS 1-8 GA 288VG J9 HYPERFINE INTERACTIONS UT ISI:000085584700008 ER PT J AU Siddons, DP Bergmann, U Hastings, JB TI Polarization effects in resonant nuclear scattering SO HYPERFINE INTERACTIONS NR 52 AB Polarization phenomena are present in every radiative transition, whether it is of atomic or nuclear origin. Nuclear resonant scattering of synchrotron radiation is an ideal technique for their study because (a) the probing radiation is in a well characterized polarization state, in most cases linear, (b) the scattered radiation can be efficiently analyzed with polarization filters, and (c) synchrotron pulses are very short compared to the lifetime of a nuclear resonance, resulting in a clean signal. In the following article we describe experimental and theoretical studies of the 14.4 keV Mossbauer resonance of Fe-57 and its transitions with linear and circular polarization. After introducing the required instrumentation a formalism to calculate time dependent polarization phenomena is derived. With the help of different scattering geometries we illustrate various aspects, such as polarization mixing and selective excitation of subsets of the resonance. Perhaps the most fascinating example is the Faraday geometry where the E-vector rotates several 360 degrees turns during the lifetime of the resonant scattering. A comparison of this phenomenon with the optical Faraday effect is given. New powerful synchrotron radiation sources will enable researchers to exploit polarization phenomena in nuclear resonant scattering to detect subtle changes in physically and chemically relevant systems. 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PY 1999 VL 123 IS 1-8 GA 288VG J9 HYPERFINE INTERACTIONS UT ISI:000085584700024 ER PT J AU Shvyd'ko, YV TI Nuclear resonance forward scattering of x rays: Time and space picture SO PHYSICAL REVIEW B NR 55 CR AFANASEV AM, 1964, ZH EKSP TEOR FIZ+, V18, P1139 AKHIEZER AI, 1965, QUANTUM ELECTRODYNAM ALEKSANDROV PA, 1975, SOV PHYS JETP, V40, P360 ALLEN L, 1975, OPTICAL RESONANCE 2 BERESTETSKII VB, 1971, RELATIVISTIC QUANTUM BLUM K, 1981, DENSITY MATRIX THEOR BLUME M, 1968, PHYS REV, V171, P417 BLUME M, 1967, PHYS REV, V165, P446 BURNHAM DC, 1969, PHYS REV, V188, P667 DEAK L, 1996, PHYS REV B, V53, P6158 GERDAU E, 1986, PHYS REV LETT, V57, P1141 GERDAU E, 1994, RESONANT ANOMALOUS X, P589 HAAS M, 1997, PHYS REV B, V56, P14082 HANNON JP, 1969, PHYS REV, V186, P306 HASTINGS JB, 1991, PHYS REV LETT, V66, P770 KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 KAGAN Y, 1973, Z NATURFORSCH A, VA 28, P1351 KIKUTA S, 1994, HYPERFINE INTERACT, V90, P335 KOHN VG, 1995, J PHYS-CONDENS MAT, V7, P7589 LANDAU LD, 1970, QUANTUM MECH NONRELA LAUBEREAU A, 1978, REV MOD PHYS, V50, P607 LEUPOLD O, 1998, HYPERFINE INTERACT, V113, P81 LYNCH FJ, 1960, PHYS REV, V120, P513 MARADUDIN AA, 1971, THEORY LATTICE DYNAM MESSIAH A, 1962, QUANTUM MECH, V2 MITSUI T, 1997, JPN J APPL PHYS 1, V36, P6525 ROHLSBERGER R, 1997, HASYLAB, P933 ROHLSBERGER R, UNPUB ROHLSBERGER R, 1997, UNPUB HASYLAB ANN RE, P933 SEPIOL B, 1996, PHYS REV LETT, V76, P3220 SHVYDKO YV, 1994, EUROPHYS LETT, V26, P215 SHVYDKO YV, 1993, EUROPHYS LETT, V22, P305 SHVYDKO YV, 1994, HYPERFINE INTERACT, V90, P287 SHVYDKO YV, 1993, J PHYS-CONDENS MAT, V5, P1557 SHVYDKO YV, 1992, J PHYS-CONDENS MAT, V4, P2663 SHVYDKO YV, 1991, JETP LETT+, V53, P69 SHVYDKO YV, 1991, JETP LETT+, V53, P231 SHVYDKO YV, 1998, PHYS REV B, V57, P3552 SHVYDKO YV, 1996, PHYS REV B, V54, P14942 SHVYDKO YV, 1995, PHYS REV B, V52, PR711 SHVYDKO YV, 1996, PHYS REV LETT, V77, P3232 SINGWI KS, 1960, PHYS REV, V120, P1093 SMIRNOV GV, 1996, HYPERFINE INTERACT, V97-8, P551 SMIRNOV GV, 1996, HYPERFINE INTERACT, V97, P51 SMIRNOV GV, 1998, PHYS REV B, V57, P5788 SMIRNOV GV, 1995, PHYS REV B, V52, P3356 SMIRNOV GV, 1996, PHYS REV LETT, V77, P183 STURHAHN W, 1994, PHYS REV B, V49, P9285 TAKAGI S, 1962, ACTA CRYSTALLOGR, V15, P1311 TRAMMELL GT, 1962, PHYS REV, V126, P1045 TRAMMELL GT, 1979, PHYS REV B, V19, P3835 TRAMMELL GT, 1978, PHYS REV B, V18, P165 VANBURCK U, 1992, PHYS REV B, V46, P6207 VANHOVE L, 1955, PHYS REV, V55, P190 WINKLER H, 1998, HYPERFINE INTERACT, V113, P443 TC 6 BP 9132 EP 9143 PG 12 JI Phys. Rev. B PY 1999 PD APR 1 VL 59 IS 14 GA 186WT J9 PHYS REV B UT ISI:000079754300018 ER PT J AU Korecki, P Korecki, J Karas, W TI Holography with gamma rays: Simulations versus experiment for alpha-Fe-57 SO PHYSICAL REVIEW B-CONDENSED MATTER NR 43 AB The gamma-ray holography was recently applied [P. Korecki et al., Phys. Rev. Lett. 79, 3518 (1997)] to image the three- dimensional structure of alpha-Fe-57 with an atomic resolution. A simple theory of the hologram formation based on single- scattering cluster formalism taking into account the polarization effects in the resonant nuclear scattering and absorption processes is presented. The high quality of the real-space reconstruction is demonstrated, however, problems arising from the cancellation of real twin images are revealed. The realistic simulations are in a good agreement with the experiment. A method for elimination of the real and twin images cancellation taking advantage of the strong dependence of the scattering phase on the detuning from the resonance in the nuclear scattering is proposed. [S0163-1829(99)03109-4]. CR ADAMS B, 1998, PHYS REV B, V57, P7526 AVANASEV AM, 1965, ZH EKSP TEOR FIZ, V48, P327 BARTON JJ, 1990, J ELECTRON SPECTROSC, V51, P37 BARTON JJ, 1991, PHYS REV LETT, V67, P3106 BARTON JJ, 1988, PHYS REV LETT, V61, P1356 BLACK PJ, 1964, P PHYS SOC LOND, V83, P925 BLUME M, 1968, PHYS REV, V171, P417 BORRMANN G, 1950, Z PHYS, V127, P297 CHAMPENEY DC, 1979, REP PROG PHYS, V42, P1017 FADLEY CS, 1990, SYNCHROTRON RAD RES GABOR D, 1948, NATURE, V161, P777 GOG T, 1995, PHYS REV B, V51, P6761 GOG T, 1996, PHYS REV LETT, V76, P3132 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1968, PHYS REV, V169, P315 HANNON JP, 1974, PHYS REV B, V9, P2791 HANNON JP, 1974, PHYS REV B, V9, P2810 HANNON JP, 1994, RESONANT ANOMALOUS X HARP GR, 1991, J ELECTRON SPECTROSC, V57, P331 HARP GR, 1990, PHYS REV LETT, V65, P1012 HERMAN GS, 1992, PHYS REV LETT, V68, P650 HOY GR, 1997, J PHYS-CONDENS MAT, V9, P8749 KAGAN Y, 1973, Z NATURFORSCH A, VA 28, P1351 KORECKI P, 1997, PHYS REV LETT, V79, P3518 KOSSEL W, 1935, Z PHYS, V94, P139 LEE LY, 1972, PHYS REV C, V6, P836 LEN PM, 1997, PHYS REV B, V55, PR3323 LEN PM, 1994, PHYS REV B, V50, P11275 MARCHESINI S, 1998, SOLID STATE COMMUN, V105, P685 MILLER GA, 1997, PHYS REV B, V56, P2399 MOSSBAUER RL, 1981, MOSSBAUER SPECTROSCO, V2 ROSE ME, 1957, ELEMENTARY THEORY AN SALDIN DK, 1990, PHYS REV LETT, V64, P1270 SLEZAK T, IN PRESS J MAGN MAGN SMIRNOV GV, 1985, ZH EKSP TEOR FIZ+, V89, P1169 STURHAHN W, 1994, PHYS REV B, V49, P9285 SZOKE A, 1986, AIP C P, V147, P361 TEGZE M, 1991, EUROPHYS LETT, V16, P41 TEGZE M, 1996, NATURE, V380, P49 TONG SY, 1992, PHYS REV B, V46, P2452 TONNER BP, 1991, PHYS REV B, V43, P14423 TRAMMELL GT, 1962, PHYS REV, V126, P1045 VOOGT FC, 1995, SURF SCI, V331, P1508 TC 4 BP 6139 EP 6152 PG 14 JI Phys. Rev. B-Condens Matter PY 1999 PD MAR 1 VL 59 IS 9 GA 178EX J9 PHYS REV B-CONDENSED MATTER UT ISI:000079254300030 ER PT J AU Sturhahn, W Alp, EE Toellner, TS Hession, P Hu, M Sutter, J TI Introduction to nuclear resonant scattering with synchrotron radiation SO HYPERFINE INTERACTIONS NR 34 AB The concepts leading to the application of synchrotron radiation to elastic and inelastic nuclear resonant scattering are discussed. The resulting new experimental techniques are compared to conventional Mossbauer spectroscopy. A survey of situations that favor experiments with synchrotron radiation is offered. CR AFANASEV AM, 1965, ZH EKSP TEOR FIZ, V21, P215 ALP EE, 1994, HYPERFINE INTERACT, V90, P323 ALP EE, 1995, NUCL INSTRUM METH B, V97, P526 BARON AQR, 1994, NUCL INSTRUM METH A, V343, P517 BLUME M, 1968, PHYS REV, V171, P417 CHUMAKOV AI, 1995, EUROPHYS LETT, V30, P427 CHUMAKOV AI, 1996, NUCL INSTRUM METH A, V383, P642 CHUMAKOV AI, 1996, PHYS REV B, V54, PR9596 FAIGEL G, 1987, PHYS REV LETT, V58, P2699 FULTZ B, 1997, PHYS REV LETT, V79, P937 GERDAU E, 1985, PHYS REV LETT, V54, P835 GERDAU E, 1994, RESONANT ANOMALOUS X HANNON JP, 1968, PHYS REV, V169, P315 HASTINGS JB, 1991, PHYS REV LETT, V66, P770 KAGAN Y, 1968, ZH EKSP TEOR FIZ, V27, P819 KISHIMOTO S, 1992, REV SCI INSTRUM, V63, P824 LIPKIN HJ, 1995, PHYS REV B, V52, P10073 MARGULIES S, 1961, NUCL INSTRUM METHODS, V12, P131 METGE J, 1990, NUCL INSTRUM METH A, V292, P187 MOONEY TM, 1994, NUCL INSTRUM METH A, V347, P348 RUBY SL, 1974, J PHYS-PARIS, V35, P209 RUFFER R, 1996, HYPERFINE INTERACT, V97-8, P589 SETO M, 1995, PHYS REV LETT, V74, P3828 SINGWI KS, 1960, PHYS REV, V120, P1093 SMIRNOV GV, 1997, AIP C P, V389, P323 SMIRNOV GV, 1996, HYPERFINE INTERACT, V97-8, P551 STURHAHN W, 1995, PHYS REV LETT, V74, P3832 STURHAHN W, 1996, REV SCI INSTRUM, V67 TOELLNER TS, 1997, APPL PHYS LETT, V71, P2112 TOELLNER TS, 1995, APPL PHYS LETT, V67, P1993 TOELLNER TS, 1994, NUCL INSTRUM METH A, V350, P595 TOELLNER TS, 1997, UNPUB VANBURCK U, 1990, EUROPHYS LETT, V13, P371 VISSCHER WM, 1960, ANN PHYS, V9, P194 TC 3 BP 47 EP 58 PG 12 JI Hyperfine Interact. PY 1998 VL 113 IS 1-4 GA 124CT J9 HYPERFINE INTERACTIONS UT ISI:000076164300005 ER PT J AU Tsinoev, VG Cherepanov, VM Rogov, EV Vidyakin, GS Shtanov, VI TI Search for P and CP violation in the M1 transition of Sn-119 with Mossbauer polarimetry technique SO PHYSICS OF ATOMIC NUCLEI NR 15 AB The ratio of the reduced matrix elements of the P-, T-odd and P-odd potentials of nucleon-nucleon interaction is measured by the Mossbauer and Compton polarimetry techniques. The results is [V-P,V-T]/[V-P]= -(1.6 +/- 4.1) x 10(-2). A SnS single crystal with a quadrupolarly split Mossbauer spectrum is used as a resonance filter-polarizer to reveal the P-odd circular polarization P-c and the P-, T-odd linear polarization P of the Mossbauer Mi-transition of Sn-119 with E = 23.8 keV. CR AFANASEV VM, 1970, PHYS LETT A, V31, P38 BALUEV AV, 1986, JETP LETT+, V43, P656 BLUME M, 1968, PHYS REV, V171, P417 DAVIS BR, 1980, PHYS REV C, V22, P1233 GOLDWIRE HC, 1977, PHYS REV B, V16, P1875 HANNON JP, 1968, PHYS REV LETT, V21, P726 HERCZEG P, 1988, HYPERFINE INTERACT, V43, P77 INZHECHIK LV, 1986, SOV J NUCL PHYS+, V44, P890 JACOBS JP, 1995, PHYS REV A, V52, P3521 KHRIPLOVICH IB, 1991, PARITY NONCONSERVATI LLOYD SP, 1951, PHYS REV, V81, P161 MURDOCH BT, 1974, PHYS LETT B, VB 52, P325 PENDLEBURY JM, 1993, ANNU REV NUCL PART S, V43, P687 POSTMA H, 1988, HYPERFINE INTERACT, V43, P120 SZYMANSKI Z, 1968, NUCL PHYS A, V113, P385 TC 1 BP 1255 EP 1260 PG 6 JI Phys. Atom. Nuclei PY 1998 PD AUG VL 61 IS 8 GA 123PE J9 PHYS ATOM NUCL-ENGL TR UT ISI:000076132900003 ER PT J AU Haas, M Realo, E Winkler, H MeyerKlaucke, W Trautwein, AX Leupold, O Ruter, HD TI Nuclear resonant forward scattering of synchrotron radiation by randomly oriented iron complexes which exhibit nuclear Zeeman interaction SO PHYSICAL REVIEW B-CONDENSED MATTER NR 18 AB An expression for the amplitude of a pulse of synchrotron radiation (SR) coherently scattered in forward direction by a randomly oriented Mossbauer absorber is derived from the theory of gamma optics. It is assumed that the hyperfine splittings present in the Mossbauer nuclei can be described in the framework of the spin-Hamiltonian formalism. In the general case of a thick Mossbauer sample, which consists of randomly oriented paramagnetic iron-containing molecules (for example, a frozen solution of a Fe-57 protein) in an applied magnetic field, the response of this sample on an incident monochromatic and fully polarized SR beam cannot be given analytically because of the integrations involved. The way to evaluate nuclear forward-scattering spectra for this general case numerically is outlined and results of calculations with a corresponding program package called SYNFOS are shown and compared with experimental results obtained by measurements of the high-spin iron (II) ''picket-fence'' porphyrin [Fe(CH3COO)TPpivP](-) in an applied field of 6 T. CR ABRAGAM A, 1951, P ROY SOC LOND A MAT, V205, P135 AFANASEV AM, 1965, ZH EKSP TEOR FIZ, V21, P215 ALP EE, 1995, NUCL INSTRUM METH B, V97, P526 BLUME M, 1968, PHYS REV, V171, P417 BOMINAAR EL, 1992, INORG CHEM, V31, P1845 DEAK L, 1996, PHYS REV B, V53, P6158 EDMONDS AR, 1957, ANGULAR MOMENTUM QUA GERDAU E, 1994, RESONANT ANOMALOUS X, P589 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1968, PHYS REV, V169, P315 HASTINGS JB, 1991, PHYS REV LETT, V66, P770 KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 KNESE K, 1995, THESIS U LEIPZIG LEUPOLD O, 1996, ITAL PHY SO, V50, P857 LEUPOLD O, UNPUB REALO E, 1996, ITAL PHY SO, V50, P861 STURHAHN W, 1994, PHYS REV B, V49, P9285 TRAUTWEIN AX, 1991, STRUCT BOND, V78, P1 TC 11 BP 14082 EP 14088 PG 7 JI Phys. Rev. B-Condens Matter PY 1997 PD DEC 1 VL 56 IS 21 GA YJ879 J9 PHYS REV B-CONDENSED MATTER UT ISI:A1997YJ87900082 ER PT J AU Sadykov, EK Isavnin, AG Skvortsov, AI TI Mossbauer transition dynamics in conditions of strong excitation of nuclear spins SO HYPERFINE INTERACTIONS NR 48 AB The state of the art Mossbauer spectroscopy has made unquestionable advance possible in the solid microstructure study. Apart from that application of the Mossbauer effect, another domain of investigations has been outlined since the outset, in the sixties, wherein the properties of gamma- radiation interaction with resonant nuclei in a recoilless mode are stressed. There were these recoilless processes that enabled to distinguish the gamma-radiation of natural width, and greatly encouraged the arising of traditional optics problems in the gamma range. The subject of interest in this article deals as well with the Mossbauer gamma optics. Essentially it is a gamma-ray (Mossbauer) susceptibility of the excited, non-equilibrium state of the nuclear spin system. We analyze the Mossbauer transitions in the strong coherent excitation of nuclear spins regime and the possibilities to deliberately vary the polarization, spectral and/or temporal properties of gamma-radiation propagating through a time- modulated medium. CR AFANASEV AM, 1980, N33379 I AT EN, P25 ANDREEVA MA, 1982, MOSSBAUER GAMMA OPTI, P226 AUTLER S, 1965, PHYS REV, V100, P703 BALDOCHIN YV, 1972, JETF, V63, P708 BASHKIROV SS, 1975, FIZ TVERD TELA+, V17, P1864 BASHKIROV SS, 1981, IZV VYSSH UCHEBN ZAV, V9, P111 BASHKIROV SS, 1979, PHYS STATUS SOLIDI B, V93, P437 BLUME M, 1968, PHYS REV, V171, P417 COUSSEMENT R, 1993, PHYS REV LETT, V71, P1824 DZYUBLIK AY, 1996, PHYS STATUS SOLIDI B, V194, P699 DZYUBLIK AY, 1981, PHYS STATUS SOLIDI B, V104, P81 GABRIEL H, 1969, PHYS REV, V184, P359 HACK MN, 1961, NUOVO CIMENTO, V19, P546 HARTMANNBOUTRON F, 1972, J PHYS-PARIS, V33, P285 IKONEN E, 1988, PHYS REV B, V38, P6380 IKONEN E, 1988, PHYS REV LETT, V60, P643 JULIAN SR, 1988, PHYS REV B, V38, P4394 KOPCEWICZ M, 1980, J PHYS CHEM SOLIDS, V91, P631 MITIN AV, 1967, JEFT, V52, P1596 MITIN AV, 1981, PHYS LETT A, V84, P278 MITIN AV, 1974, PHYS LETT A, V49, P1111 MONAHAN JE, 1979, PHYS REV A, V20, P1499 OLARIU S, 1986, EUROPHYS LETT, V2, P725 OLARIU S, 1994, PHYS REV B, V50, P43 OLARIU S, 1994, PHYS REV B, V50, P616 OLARIU S, 1988, PHYS REV B, V37, P7698 PERLOW GJ, 1968, PHYS REV, V172, P319 PERLOW GJ, 1978, PHYS REV LETT, V40, P896 PFEIFFER L, 1971, J APPL PHYS, V42, P1725 PFEIFFER L, 1972, PHYS REV B-SOLID ST, V6, P74 RUBY SL, 1960, PHYS REV LETT, V50, P5 SADYKOV EK, 1994, FIZ TVERD TELA+, V36, P3473 SADYKOV EK, 1991, FIZ TVERD TELA+, V33, P2725 SADYKOV EK, 1987, FIZ TVERD TELA+, V29, P3162 SADYKOV EK, 1990, PHYS STATUS SOLIDI B, V158, P685 SADYKOV EK, 1989, PHYS STATUS SOLIDI B, V156, P605 SADYKOV EK, 1984, PHYS STATUS SOLIDI B, V123, P703 SADYKOV EK, 1993, THESIS KAZAN SALKOLA M, 1990, PHYS REV A, V41, P3838 SINOR TW, 1989, PHYS REV LETT, V62, P2547 SJAVAVKO MS, 1986, DOKL AKAD NAUK SSSR, V292, P1065 SMIRNOV GV, 1986, HYPERFINE INTERACT, V27, P203 SMIRNOV GV, 1984, ZH EKSP TEOR FIZ+, V86, P1495 SRIVASTAVA JK, 1983, ADV MOSSBAUER SPECTR, P761 TITTONEN I, 1993, HYPERFINE INTERACT, V78, P397 TITTONEN I, 1992, PHYS REV LETT, V69, P2815 VAGIZOV FG, 1990, HYPERFINE INTERACT, V61, P1359 VOITOVETSK BK, 1984, N39522 I AT EN, P52 TC 2 BP 257 EP 275 PG 19 JI Hyperfine Interact. PY 1997 VL 107 IS 1-4 GA XE449 J9 HYPERFINE INTERACTIONS UT ISI:A1997XE44900022 ER PT J AU Hoy, GR TI Time-domain, nuclear-resonant, forward scattering: The classical approach SO HYPERFINE INTERACTIONS NR 24 AB This paper deals with the interaction of electromagnetic radiation with matter assuming the matter to have nuclear transitions in resonance with incident electromagnetic radiation. The source of the radiation is taken to be of two types; natural radioactive gamma decay and synchrotron radiation. Numerical examples using Fe-57 are given for the two types of source radiation. Calculated results are contrasted for the two cases. Electromagnetic radiation produced by recoil-free gamma-ray emission has essentially the natural linewidth. Electromagnetic radiation from a synchrotron, even with the best monochromators available, has a relatively broad- band spectrum, essentially constant for these considerations. Polarization effects are considered. In general, the nuclear- resonant medium changes the polarization of the input radiation on traversing the medium. Calculations are presented to illustrate that synchrotron radiation studies using nuclear- resonant forward scattering have the potential for making high- precision measurements of hyperfine fields and recoilless fractions. An interesting aspect of nuclear-resonant forward scattering, relative to possible gamma-ray laser development, is the so-called ''speed-up'' effect. CR BERGMAN U, 1994, THESIS STATE U NEW Y, P33 BLATT JM, 1952, THEORETICAL NUCLEAR BLUME M, 1968, PHYS REV, V171, P417 DICKE RH, 1954, PHYS REV, V93, P99 FOLDY LL, 1945, PHYS REV, V67, P107 GERDAU E, 1986, PHYS REV LETT, V57, P1141 GERDAU E, 1985, PHYS REV LETT, V54, P835 HAMILL DW, 1968, PHYS REV LETT, V21, P724 HANNON JP, 1969, PHYS REV, V186, P306 HARRIS SM, 1961, PHYS REV, V124, P1178 HOLLAND RE, 1960, PHYS REV LETT, V4, P181 HOY GR, 1992, ENCY PHYSICAL SCI TE, V10, P469 HOY GR, 1972, PHYS REV LETT, V28, P877 LAX M, 1951, REV MOD PHYS, V23, P287 LYNCH FJ, 1960, PHYS REV, V120, P513 MOSSBAUER RL, 1968, PHYS LETT A, V28, P94 MOSSBAUER RL, 1958, Z PHYS, V151, P124 NEUWIRTH W, 1966, Z PHYS, V197, P473 STURHAHN W, 1994, PHYS REV B, V49, P9285 TRIFTSHAUSER W, 1967, PHYS REV, V162, P274 TRIFTSHAUSER W, 1966, PHYS REV LETT, V16, P1161 VANBURCK U, 1994, HYPERFINE INTERACT, V19, P313 VANBURCK U, 1992, PHYS REV B, V46, P6207 WU CS, 1960, PHYS REV LETT, V5, P432 TC 0 BP 381 EP 399 PG 19 JI Hyperfine Interact. PY 1997 VL 107 IS 1-4 GA XE449 J9 HYPERFINE INTERACTIONS UT ISI:A1997XE44900032 ER PT J AU Pinoev, VG Cherepanov, VM Baluev, AV Mityakhina, VS Antipov, AA TI Mossbauer polarimeter for the experiment on the search of space parity disorder in dysprosium-161 SO FIZIKA TVERDOGO TELA NR 11 CR ANTIPOV AA, 1984, 3 VSES SOV SPEKTR KO, P109 BALUEV AV, 1985, APPL MOSSBAUER EFFEC, V2 BALUEV AV, 1986, PISMA ESKP TEOR FIZ, V43, P507 BANDURKIN IA, 1984, OSOBENNOSTI KRISTALL BLUME M, 1968, PHYS REV, V171, P417 FRAUENFELDER H, 1962, PHYS REV, V126, P1065 IMBERT P, 1966, J PHYS, V27, P429 INZHECHIK LV, 1990, YAF, V51, P14 INZHECHIK LV, 1987, ZH EKSP TEOR FIZ+, V93, P1569 MITYAKHINA VS, 1986, THESIS RADIEVYI I VG TSINOEV VG, 1992, INT S WEAK ELECT INT TC 0 BP 3022 EP 3028 PG 7 JI Fiz. Tverd. Tela PY 1996 PD OCT VL 38 IS 10 GA VZ297 J9 FIZ TVERD TELA UT ISI:A1996VZ29700017 ER PT J AU Deak, L Bottyan, L Nagy, DL Spiering, H TI Coherent forward-scattering amplitude in transmission and grazing incidence Mossbauer spectroscopy SO PHYSICAL REVIEW B-CONDENSED MATTER NR 19 AB The theory of both transmission and grazing incidence Mossbauer spectroscopy is reanalyzed. Starting with the nuclear susceptibility tensor a common concise first-order perturbation formulation is given by introducing the forward-scattering amplitude into an anisotropic optical scheme. Formulas of Blume and Kistner as well as those of Andreeva are rederived for the forward-scattering and grazing incidence geometries, respectively. Limitations of several previously intuitively introduced approximations are pointed out. The grazing incidence integral propagation matrices are written in a form built up from 2 x 2 matrix exponentials which is particularly suitable for numerical calculations and practical fitting of both energy domain (conventional source experiment) and time domain (synchrotron radiation experiment) Mossbauer spectra. CR AFANASEV AM, 1965, ZH EKSP TEOR FIZ, V21, P215 ANDREEVA MA, 1982, MESSBAUEROVSKAYA GAM ANDREEVA MA, 1986, POVERKHNOST, V9, P145 ANDREEVA MA, 1994, SOV PHYS JETP, V78, P965 ANDREEVA MA, 1986, VESTN MOSK U FIZ AS+, V27, P57 BLUME M, 1968, PHYS REV, V171, P417 BORZDOV GN, 1976, ZH PRIKL SPEKTROSK, V25, P526 FEDOROV FI, 1976, TEORIYA GIROTROPII FORST JC, 1985, APPL PHYS LETT, V47, P581 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1968, PHYS REV, V169, P315 HANNON JP, 1985, PHYS REV B, V32, P5068 HANNON JP, 1985, PHYS REV B, V32, P6363 IRKAEV SM, 1993, NUCL INSTRUM METH B, V74, P545 IRKAEV SM, 1993, NUCL INSTRUM METH B, V74, P554 LAX M, 1951, REV MOD PHYS, V23, P287 NAGY DL, 1992, HYPERFINE INTERACT, V71, P1349 ROHLSBERGER R, 1994, THESIS U HAMBURG SPIERING H, 1985, HYPERFINE INTERACT, V24, P737 TC 11 BP 6158 EP 6164 PG 7 JI Phys. Rev. B-Condens Matter PY 1996 PD MAR 1 VL 53 IS 10 GA TZ773 J9 PHYS REV B-CONDENSED MATTER UT ISI:A1996TZ77300030 ER PT J AU BERGMANN, U TI MOSSBAUER-SPECTROSCOPY WITH SYNCHROTRON-RADIATION SO APPLIED RADIATION AND ISOTOPES NR 29 AB Synchrotron radiation is an attractive source for Mossbauer spectroscopy because of its unique properties, such as, short pulse nature, large brightness, well-defined polarization and high collimation. Due to the delta-pulse excitation of the nuclear resonance, the intensity of the subsequent decay is measured energy integrated as a function of time, instead of time integrated as a function of energy (source/absorber velocity), like in a conventional Mossbauer experiment. The resulting time spectrum contains the full information of the Mossbauer parameters and is essentially source independent. Thus, in contrast to the conventional technique, source related complications in the data analysis are completely removed. In addition, the well-defined polarization of the SR-pulse facilitates the analysis in general and the study of polarization phenomena in particular. Two examples, namely the measurements of the temperature dependence and polarization mixing of forward scattering from alpha-Fe-57 nuclei are presented. CR ALP EE, 1993, PHYS REV LETT, V70, P3351 BERGMANN U, 1995, HYPERFINE INT P ICAM BERGMANN U, 1994, PHYS REV B, V50, P5957 BERGMANN U, 1994, RESONANT ANOMALOUS X BERGMANN U, 1994, THESIS STATE U NEW Y BLUME M, 1968, PHYS REV, V171, P417 GERDAU E, 1985, PHYS REV LETT, V54, P835 GERDAU E, 1994, RESONANT ANOMALOUS X HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1973, PHYS REV B, V9, P2810 HASTINGS JB, 1991, PHYS REV LETT, V66, P770 HECHT E, 1989, OPTICS KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 MALMFORS KB, 1952, ARK FYS, V6, P49 MOON PB, 1951, P PHYS SOC A, V64, P76 MOSSBAUER RL, 1958, NATURWISSENSCHAFTEN, V45, P538 MOSSBAUER RL, 1958, Z PHYS, V151, P124 MULLEN JG, 1988, PHYS REV B, V37, P3226 POUND RV, 1960, PHYS REV LETT, V4, P337 ROHLSBERGER R, 1994, THESIS U HAMBURG RUBY SL, 1974, J PHYS-PARIS, V35, P209 SEPPI EJ, 1962, PHYS REV, V128, P2334 SIDDONS DP, 1993, PHYS REV LETT, V70, P359 SIDDONS DP, 1990, PHYS REV LETT, V64, P1967 STURHAHN W, 1991, EUROPHYS LETT, V14, P821 TRAMMELL GT, 1979, PHYS REV B, V19, P3835 TRAMMELL GT, 1978, PHYS REV B, V18, P165 VANBURCK U, 1992, PHYS REV B, V46, P6207 YU K, 1973, Z NATURFRSCH A, V28, P1351 TC 1 BP 525 EP 530 PG 6 JI Appl. Radiat. Isot. PY 1995 PD JUN-JUL VL 46 IS 6-7 GA RJ946 J9 APPL RADIAT ISOTOPES UT ISI:A1995RJ94600053 ER PT J AU ANDRIYANCHIK, AA BARYSHEVSKY, VG KAMINSKY, AN TI GRAZING-INCIDENCE X-RAY-DIFFRACTION IN CRYSTALS WITH MAGNETIC AMORPHOUS FILM SO PHYSICA STATUS SOLIDI A-APPLIED RESEARCH NR 10 AB Grazing-incidence diffraction on crystals with an amorphous magnetic layer is considered. It is shown that even far from the absorption lines, when the difference between the refractive indices for the waves with different polarizations is small, this diffraction geometry can be effectively used for the investigation of thin magnetic films. The effect of the excitation of waves with orthogonal polarization is analyzed when a wave with the eigen-polarization is incident on the surface of the magnetic film. Results of numerical calculations are given for X-ray diffraction on a germanium single crystal with an amorphous magnetic layer. CR ALEKSANDROV PA, 1984, PHYS STATUS SOLIDI A, V81, P47 ANDREYEV AV, 1985, USP FIZ NAUK+, V145, P113 ANDREYEVA MA, 1985, KRISTALLOGRAFIYA+, V30, P849 ANDRIYANCHIK AA, 1994, PHYS STATUS SOLIDI A, V142, P315 BARYSHEVSKY VG, 1976, NUCLEAR OPTICS POLAR BLUME M, 1968, PHYS REV, V171, P417 GOEDKOOP JB, 1988, PHYS REV B, V37, P2086 HANNON JP, 1988, PHYS REV LETT, V61, P1245 SCHUTZ G, 1987, PHYS REV LETT, V58, P737 THOLE BT, 1985, PHYS REV LETT, V55, P2086 TC 0 BP 15 EP 21 PG 7 JI Phys. Status Solidi A-Appl. Res. PY 1995 PD JAN 16 VL 147 IS 1 GA QH741 J9 PHYS STATUS SOLIDI A-APPL RES UT ISI:A1995QH74100001 ER PT J AU PERLOW, GJ PIEPER, SC TI TEMPORAL OPTICS OF RESONANT TRANSMISSION OF GAMMA-RAYS THROUGH FE-57 SO HYPERFINE INTERACTIONS NR 13 AB The development in time of the transmission through Fe-57 of a broad Lorenztian radiation is calculated numerically. Examples are given for theta=0 and pi/2, for the magnetic hyperfine case, and for theta=pi/2 for pure quadrupole splitting. CR BLUME M, 1968, PHYS REV, V171, P417 FAIGEL G, 1987, PHYS REV LETT, V58, P2699 GERDAU E, 1986, PHYS REV LETT, V57, P1141 GERDAU E, 1985, PHYS REV LETT, V54, P835 HAMERMESH M, 1960, ANL6111 REP, P6 HANNON JP, 1985, PHYS REV B, V2, P6363 KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 LYNCH FJ, 1960, PHYS REV, V120, P513 PERLOW GJ, 1992, HYPERFINE INTERACT, V72, P51 ROSE ME, 1957, ELEMENTARY THEORY AN RUFFER R, 1987, PHYS REV LETT, V58, P2359 TRAMMELL GT, 1962, PHYS REV, V126, P1045 VANBURCK U, 1987, PHYS REV LETT, V59, P355 TC 1 BP 1065 EP 1070 PG 6 JI Hyperfine Interact. PY 1994 VL 92 IS 1-4 GA QB952 J9 HYPERFINE INTERACTIONS UT ISI:A1994QB95200021 ER PT J AU PERLOW, GJ PIEPER, SC TI SIMULATION OF THE TIME-DEPENDENT FARADAY-EFFECT FOR SYNCHROTRON-RADIATION SO HYPERFINE INTERACTIONS NR 7 AB Synchrotron radiation is simulated by a broad Lorentzian in a calculation of the time-dependent Faraday effect in Fe-57. An extension of the method of Hamermesh to the multi-line case is used. CR BLUME M, 1968, PHYS REV, V171, P417 HANNON JP, 1985, PHYS REV B, V2, P6363 LAX M, 1951, REV MOD PHYS, V23, P287 PERLOW GJ, 1994, HYPERFINE INTERACT, V92, P1065 ROSE ME, 1957, ELEMENTARY THEORY AN SIDDONS DP, 1993, PHYS REV LETT, V70, P359 TRAMMELL GT, 1962, PHYS REV, V126, P1045 TC 0 BP 1071 EP 1075 PG 5 JI Hyperfine Interact. PY 1994 VL 92 IS 1-4 GA QB952 J9 HYPERFINE INTERACTIONS UT ISI:A1994QB95200022 ER PT J AU DEAK, L BOTTYAN, L NAGY, DL TI CALCULATION OF NUCLEAR RESONANT SCATTERING SPECTRA OF MAGNETIC MULTILAYERS SO HYPERFINE INTERACTIONS NR 11 AB We report on calculations of the angle- and time-dependent photon reflectivity of multilayers using the technique of characteristic matrices. Spectra of Fe-56/Fe-57 and Cr/Fe multilayers are calculated under various conditions. The parameters of the multilayers are optimized for suitable test samples of reflectometry measurements. CR BLUME M, 1968, PHYS REV, V171, P417 BORN M, 1970, PRINCIPLES OPTICS, P51 CHUMAKOV AI, 1991, PISMA ESKP TEOR FIZ, V53, P258 DEAK L, 1993, 18TH P ZAK SCH PHYS, P269 FOLKERTS W, 1992, J APPL PHYS, V71, P362 HANNON JP, 1969, PHYS REV, V186, P306 HANNON JP, 1985, PHYS REV B, V32, P5068 HANNON JP, 1985, PHYS REV B, V32, P6363 KAGAN Y, 1979, J PHYS C SOLID STATE, V12, P615 LAX M, 1951, REV MOD PHYS, V23, P287 NAGY DL, 1992, HYPERFINE INTERACT, V71, P1349 TC 8 BP 1083 EP 1088 PG 6 JI Hyperfine Interact. PY 1994 VL 92 IS 1-4 GA QB952 J9 HYPERFINE INTERACTIONS UT ISI:A1994QB95200024 ER PT J AU BERGMANN, U SIDDONS, DP HASTINGS, JB TI TIME-DEPENDENT POLARIZATION IN MOSSBAUER EXPERIMENTS WITH SYNCHROTRON-RADIATION .2. SO HYPERFINE INTERACTIONS NR 11 AB The resonant forward scattering of X-rays from Fe-57 nuclei is strongly polarization dependent. The broad band excitation provided by synchrotron radiation (SR) results in an interesting time-dependent polarization mixing. This mixing can be used to substantially reduce the nonresonant (nonrotated) scattering from electrons. The presented technique will allow the full utilization of next-generation synchrotron facilities as a source for Mossbauer experiments. CR 1989, OPTICS BERGMANN U, IN PRESS P INT C ANO BLUME M, 1968, PHYS REV, V171, P417 GERDAU E, UNPUB P INT C ANOMAL HANNA SS, 1960, PHYS REV LETT, V4, P177 HANNON JP, 1990, COMMUNICATION HANNON JP, 1969, PHYS REV, V186, P306 KAGAN Y, 1973, Z NATURFORSCH A, VA 28, P1351 SIDDONS DP, 1993, PHYS REV LETT, V70, P359 SIDDONS DP, 1990, PHYS REV LETT, V64, P1967 TRAMMELL GT, 1978, PHYS REV B, V18, P165 TC 2 BP 1113 EP 1121 PG 9 JI Hyperfine Interact. PY 1994 VL 92 IS 1-4 GA QB952 J9 HYPERFINE INTERACTIONS UT ISI:A1994QB95200029 ER PT J AU BOOLCHAND, P BRESSER, W ANAPLE, G WU, Y ENZWEILER, RN COUSSEMENT, R GROVER, J TI GAMMA-RAY POLARIZATION IN TRANSMISSION THROUGH A NONCUBIC AND NONMAGNETIC SINGLE-CRYSTAL SO PHYSICAL REVIEW B-CONDENSED MATTER NR 14 AB A Mossbauer-effect experiment, with gamma-ray wave vector k directed both along and normal to the c axis of a siderite (FeCO3) single-crystal platelet, has been systematically performed in the temperature range 50 < T < 300 K. The T dependence of the integrated area S(T) = S(pi)(T) + S(sigma)(T) under the quadrupole doublet reveals that at 300 K the Debye- Waller factors are f(c) = 0.72(2) and f(perpendicular-to c) = 0.75(2). Independently, the area ratios S(pi/S(sigma under the pi and sigma quadrupole components, measured at 300 K, confirm the lack of a spatial anisotropy of the f factor but, more significantly, confirm the theoretically predicted polarization-dependent resonant-absorption cross section in transmission through the crystal. CR 1980, UNPUB MINERAL POWDER, P887 BLUME M, 1968, PHYS REV, V171, P417 BOOLCHAND P, 1970, PHYS REV B, V2, P3463 BOOLCHAND P, 1991, PHYS REV LETT, V67, P3184 BOOLCHAND P, 1969, THESIS CARE W RESERV DEER WA, 1964, ROCK FORMING MINER, V5, P273 GOLDANSKII VI, 1968, PHYS REV LETT, V20, P137 HOUSLEY RM, 1969, PHYS REV, V178, P514 HOUSLEY RM, 1968, PHYS REV LETT, V20, P1279 OK HN, 1969, PHYS REV, V185, P475 OKIJI A, 1964, J PHYS SOC JPN, V19, P908 ONO K, 1964, J PHYS SOC JPN, V19, P899 SHARP WE, 1960, AM MINERAL, V45, P241 TRAMMELL GT, 1962, PHYS REV, V126, P1045 TC 0 BP 6833 EP 6839 PG 7 JI Phys. Rev. B-Condens Matter PY 1994 PD SEP 1 VL 50 IS 10 GA PH222 J9 PHYS REV B-CONDENSED MATTER UT ISI:A1994PH22200034 ER PT J AU DUNHAM, WR HARDING, LJ SANDS, RH TI MOSSBAUER-SPECTROSCOPY OF METALLOPROTEINS AND THE USE OF FOURIER-TRANSFORMS SO EUROPEAN JOURNAL OF BIOCHEMISTRY NR 15 AB A method for obtaining accurate, quantitative Fe-57 Mossbauer spectra from biological samples is illustrated stepwise in a data reduction procedure. Exact criteria are presented for deciding when it is necessary to account for the effects of the Beer-Lambert law in the Mossbauer spectra from biological samples. This procedure makes extensive use of the fast Fourier transform and other computer techniques in its data reduction and its curve-fitting stages. A method for optimizing sample thickness is presented. The choice of truncation in Fourier space as a means to numerically stabilize the deconvolution procedure is defended. Several advantages for curve fitting in Fourier space are shown. Maximization of information content is discussed for Mossbauer spectral simulation techniques. CR BLUME M, 1968, PHYS REV, V171, P417 DEBENEDETTI S, 1966, ANN REV NUCL SCI, V16, P31 DUNHAM WR, 1985, EUR J BIOCHEM, V146, P497 DUNHAM WR, 1980, J MAGN RESON, V40, P351 DUNHAM WR, 1977, NUCL INSTRUM METHODS, V145, P537 EVANS RD, 1955, ATOMIC NUCLEUS, P711 EVANS RD, 1955, ATOMIC NUCLEUS, P785 FILTER WF, 1978, FRONTIERS BIOL ENERG, V1, P603 FILTER WF, 1983, THESIS U MICHIGAN FRAUENFELDER H, 1962, MOSSBAUER EFFECTS GREENWOOD NN, 1971, MOSSBAUER SPECTROSCO GRODSTEIN GW, 1957, NBS583 CIRC WASH HOUSLEY RM, 1965, NUCL INSTRUM METHODS, V35, P77 URE MCD, 1971, MOSSBAUER EFFECT MET, V7, P245 WU CT, 1975, THESIS U MICHIGAN TC 4 BP 1 EP 8 PG 8 JI Eur. J. Biochem. PY 1993 PD MAY 15 VL 214 IS 1 GA LE436 J9 EUR J BIOCHEM UT ISI:A1993LE43600001 ER PT J AU IRKAEV, SM ANDREEVA, MA SEMENOV, VG BELOZERSKII, GN GRISHIN, OV TI GRAZING-INCIDENCE MOSSBAUER-SPECTROSCOPY - NEW METHOD FOR SURFACE-LAYERS ANALYSIS .2. THEORY OF GRAZING-INCIDENCE MOSSBAUER-SPECTRA SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B- BEAM INTERACTIONS WITH MATERIALS AND ATOMS NR 27 AB A general theory of grazing incidence Mossbauer spectroscopy (GIMS) spectra for an inhomogeneous layered medium is presented. The computer simulation based on this theory shows that the shape of the resonant spectrum of the reflected wave intensity, in the case of a resonant film, differs considerably from the case of a semiinfinite resonant mirror. This shape strongly depends on the thickness and the properties of the film and of the nonresonant substrate. The proposed theory of the lineshape of Mossbauer secondary radiation spectra from resonant films takes into account the influence of different types of photo- and conversion electrons on the resulting spectrum. It is shown that the fitting of grazing incidence Mossbauer spectra can be done only by means of numerical simulations. CR ALEKSANDROV PA, 1980, FIZ TVERD TELA+, V22, P2797 ANDREEVA MA, 1992, JETP LETT, V55, P62 ANDREEVA MA, 1982, MOSSBAUEROVSKAYA GAM ANDREEVA MA, 1984, OPT SPEKTROSK+, V56, P546 ANDREEVA MA, 1991, PHYS STATUS SOLIDI A, V127, P455 ANDREEVA MA, 1984, PHYS STATUS SOLIDI B, V125, P461 ANDREEVA MA, 1981, PHYS STATUS SOLIDI B, V103, P193 ANDREEVA MA, 1986, POVERKHNOST, V9, P145 ANDREEVA MA, 1986, VESTN MOSK U FIZ AS+, V27, P57 ANDREEVA MA, 1987, ZH TEKH FIZ+, V57, P2009 ANDREEVA MA, 1983, ZH TEKH FIZ+, V53, P1395 AZZAM RMA, 1977, ELLIPSOMETRY POLARIZ BEDZYK MJ, 1988, NUCL INSTRUM METH A, V266, P679 BERNSTEIN S, 1963, PHYS REV, V132, P1625 BLUME M, 1968, PHYS REV, V171, P417 BORN M, 1968, PRINCIPLES OPTICS BORZDOV GN, 1976, ZH PRIKL SPECTR, V25, P527 FROST JC, 1985, APPL PHYS LETT, V47, P581 HANNON JP, 1985, PHYS REV B, V32, P5068 HANNON JP, 1985, PHYS REV B, V32, P5081 HANNON JP, 1985, PHYS REV B, V32, P6363 HANNON JP, 1985, PHYS REV B, V32, P6374 HANNON JP, 1979, PHYS REV LETT, V43, P636 IRKAEV SM, 1993, NUCL INSTRUM METH B, V74, P545 LILJEQUIST D, 1978, NUCL INSTRUM METHODS, V155, P529 PARRATT LG, 1954, PHYS REV, V95, P359 WAGNER FE, 1968, Z PHYS, V210, P361 TC 14 BP 554 EP 564 PG 11 JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PY 1993 PD JUN VL 74 IS 4 GA LG426 J9 NUCL INSTRUM METH PHYS RES B UT ISI:A1993LG42600012 ER PT J AU YANG, XL JIAN, KY WENG, SH ZHANG, FG WU, Z HU, BY TI MOSSBAUER FARADAY-EFFECT IN FE3O4 SO SCIENCE IN CHINA SERIES A-MATHEMATICS PHYSICS ASTRONOMY NR 7 AB We have observed the Mossbauer Faraday effect in nonstoichiometric Fe3O4 by the Mossbauer polarimeter. Experimental results demonstrate that the electronic hopping above Verwey temperature within Fe2+-Fe3+ ions on the octahedral sites is only a localized phenomenon and the recoilless fractions of Fe-57 nuclei in Fe3-0.02vO4 are 0.71 for A sites and 0.62 for B sites, respectively. CR BLUME M, 1968, PHYS REV, V171, P417 DANIELS JM, 1969, J PHYS CHEM SOLIDS, V30, P1561 GONSER U, 1981, TOP APPL PHYS, P99 HOUSLEY RM, 1968, PHYS REV, V171, P480 SAWATZKY GA, 1969, PHYS REV, V183, P383 YANG XL, 1989, IEEE T MAGN, V25, P684 YANG XL, 1987, J ECNU, V3, P41 TC 0 BP 48 EP 53 PG 6 JI Sci. China Ser. A-Math. Phys. Astron. PY 1993 PD JAN VL 36 IS 1 GA KP115 J9 SCI CHINA SER A UT ISI:A1993KP11500005 ER PT J AU SIDDONS, DP BERGMANN, U HASTINGS, JB TI TIME-DEPENDENT POLARIZATION IN MOSSBAUER EXPERIMENTS WITH SYNCHROTRON RADIATION - SUPPRESSION OF ELECTRONIC SCATTERING SO PHYSICAL REVIEW LETTERS NR 16 AB The resonant, forward scattering of x rays from Fe-57 nuclei is strongly polarization dependent. The broad-band excitation provided by synchrotron radiation (SR) results in an interesting time-dependent polarization mixing, which we will discuss. Further we demonstrate that by selecting only the component of the transmitted radiation which has a 90-degrees rotated plane of polarization, the nonresonant (nonrotated) transmitted intensity can be substantially reduced. This new technique will allow full utilization of new powerful SR sources currently under construction. CR BERGMANN U, UNPUB BLUME M, 1968, PHYS REV, V171, P417 GERDAU E, 1985, PHYS REV LETT, V54, P835 GONSER U, 1968, PHYS LETT A, V26, P157 HANNA SS, 1960, PHYS REV LETT, V4, P177 HANNON JP, COMMUNICATION HANNON JP, 1969, PHYS REV, V186, P306 HASTINGS JB, 1991, PHYS REV LETT, V66, P770 HECHT E, 1989, OPTICS IMBERT P, 1964, PHYS LETT, V8 KAGAN Y, 1973, Z NATURFORSCH A, VA 28, P1351 RUBY SL, 1974, J PHYS-PARIS, V35, P209 SIDDONS DP, 1990, PHYS REV LETT, V64, P1967 SIDDONS DP, 1989, PHYS REV LETT, V62, P1384 TRAMMELL GT, 1978, PHYS REV B, V18, P165 VANBURCK U, 1992, PHYS REV B, V46, P6207 TC 25 BP 359 EP 362 PG 4 JI Phys. Rev. Lett. PY 1993 PD JAN 18 VL 70 IS 3 GA KG618 J9 PHYS REV LETT UT ISI:A1993KG61800028 ER PT J AU LINDEN, J HIETANIEMI, J IKONEN, E LIPPMAA, M TITTONEN, I KATILA, T KARLEMO, T KARPPINEN, M NIINISTO, L ULLAKKO, K TI EUROPIUM-BASED HIGH-TEMPERATURE SUPERCONDUCTORS STUDIED BY X- RAY-DIFFRACTION AND EU-151 MOSSBAUER-SPECTROSCOPY SO PHYSICAL REVIEW B-CONDENSED MATTER NR 25 AB Isotropic powders and magnetically aligned crystallites of EuBa2Cu3O7-delta (1:2:3) and europium-doped Bi2Sr2CaCu2O8 (2:2:1:2) were studied by means of x-ray diffraction and Eu-151 Mossbauer spectroscopy. The degree of crystallite orientation of the samples and the values of the lattice constants were determined by x-ray diffraction. The Mossbauer spectra were analyzed considering the full hyperfine Hamiltonian of the nuclear states of the 21.5-keV gamma transition. The Mossbauer hyperfine parameters obtained from the superconducting and semiconducting phases are presented. A small change is seen in the Eu-151 isomer shift when the oxygen deficiency delta of the 1:2:3 compound is varied. The shift can be explained by a decrease in the s-electron density due to lattice expansion. The changes in the oxidation state of the copper atoms with varying delta were determined from the Mossbauer data: The Cu(2) atoms retain their oxidation state, whereas the Cu(I) atoms adjust their valence according to the value of delta. In the 2:2:1:2 samples, the Eu concentration clearly affected the value of the electric-field gradient at the Eu nucleus. Using a standard procedure, magnetically aligned 2:2:1:2 samples were prepared. The preferred direction of the crystal c axis changed from parallel to perpendicular alignment with the external magnetic field, when the Eu concentration exceeded 20% of the Ca atoms. CR ADRIAN FJ, 1988, PHYS REV B, V38, P2426 AKIRA Y, 1990, J PHYS SOC JPN, V59, P1921 ANTSON OK, 1991, PHYSICA C, V173, P65 BHATTACHARYYA S, 1989, J MAGN MAGN MATER, V80, P276 BLOK J, 1966, PHYS REV, V143, P278 BLUME M, 1968, PHYS REV, V171, P417 DERENZI R, 1989, PHYSICA C, V162, P155 FARRELL DE, 1987, PHYS REV B, V36, P4025 FERREIRA JM, 1988, APPL PHYS A-MATER, V47, P105 FREIMUTH A, 1987, Z PHYS B CON MAT, V68, P433 GROEN WA, 1989, J LESS-COMMON MET, V155, P133 GUTLICH P, 1975, TOP APPL PHYS, V5, P62 IKONEN E, 1988, HIGH TC SUPERCONDUCT, P209 KALVIUS GM, 1974, J PHYS C SOLID STATE, V6, P139 KARPPINEN M, IN PRESS SUPERCOND S LIPPMAA M, 1989, PHYS LETT A, V139, P353 MEUFFELS P, 1988, PHYSICA C, V156, P441 NISHIDA N, 1990, PHYSICA C, V168, P23 SHENOY GK, 1981, HDB SPECTROSCOPY, P490 STADNIK ZM, 1989, PHYS REV B, V39, P9108 STERNHEIMER RM, 1963, PHYS REV, V132, P1637 STEVENS JG, 1981, HDB SPECTOSCOPY, P468 TITTONEN I, 1990, HYPERFINE INTERACT, V55, P1399 WILLIAMS A, 1988, PHYS REV B, V37, P7960 WORTMANN G, 1988, PHYS LETT A, V126, P434 TC 12 BP 8534 EP 8541 PG 8 JI Phys. Rev. B-Condens Matter PY 1992 PD OCT 1 VL 46 IS 13 GA JT040 J9 PHYS REV B-CONDENSED MATTER UT ISI:A1992JT04000069 ER PT J AU TENNANT, WC TI ANALYSIS OF SINGLE-CRYSTAL MOSSBAUER DATA IN LOW-SYMMETRY FE-57 CENTERS SO JOURNAL OF PHYSICS-CONDENSED MATTER NR 20 AB The Mossbauer single-crystal experiment is discussed with particular reference to the low-symmetry resonant sites. It is demonstrated that ambiguities associated with multiple, symmetry-related resonant sites (that is, sites whose Laue class is lower than that of the host crystal) are resolvable provided the absorber recoilless fractions can be precisely measured. A general computer program, MOSREF, is described that enables simulation of single-crystal spectra and/or refinement of Mossbauer parameters for a Fe-57 centre in a site of any known symmetry in a host crystal of any known symmetry. The procedures are illustrated for a couple of ideal examples: a triclinic site in a monoclinic crystal and a monoclinic site in a trigonal crystal. Applications to recent experiments with the sheet micas biotite and muscovite are given. 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Matter PY 1992 PD AUG 17 VL 4 IS 33 GA JK088 J9 J PHYS-CONDENS MATTER UT ISI:A1992JK08800012 ER PT J AU BROWN, DE ARTHUR, J BARON, AQR BROWN, GS SHASTRI, S TI PHASE-SHIFT OF A ROTATED QUANTUM STATE OBSERVED IN AN X-RAY- SCATTERING EXPERIMENT SO PHYSICAL REVIEW LETTERS NR 25 AB The rotation of the reference frame of a particle is known to lead to a phase change of its wave function proportional to its angular momentum. This can manifest itself as an angle- dependent phase shift of a photon scattered by a fixed target, when the photon state is an eigenstate of the component of total angular momentum perpendicular to the scattering plane. This phase shift has been observed in the quantum beat pattern resulting from the transient excitation of Fe-57 nuclei by synchrotron radiation. 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