Preparation and magnetic properties of the CoO/Co bilayer B. Raquet a, R. Mamy a*, J.C. Ousset a, N. Nègre a, M. Goiran a and C. Guerret-Piécourt b aLaboratoire de Physique de la Matière Condensée de Toulouse, INSA. SNCMP, Universite Paul sabatier, Complexe Scientifique de Rangueil, 31077 Toulouse Cedex 4, France bLAAS-CNRS, 7 av. du Colonel Roche, 31077 Toulouse Cedex, France Received 28 July 1997; Received in revised form 7 November 1997 Abstract The results of the preparation, characterization and magnetic properties of a CoO/Co interface are discussed. This interface was realized by ultraviolet irradiation of a 4nm Co layer deposited with a gold buffer layer on a GaAs(111) substrate. The Co oxide analyzed by XPS and AFM revealed a continuous 1.7nm thick layer with a rms roughness of 0.6nm and mostly CoO at the interface. Longitudinal magneto-optical Kerr loops evidence a strong initial in-plane anisotropy which disappears on oxidation. Values of the unidirectional exchange coupling at the Co/CoO interface were obtained: 0.1erg/cm2 from SQUID measurement at 5K after field cooling and 0.6erg/cm2 with magneto-optical Kerr effect in polar configuration from modelization of the M(H) curve. This discrepancy is discussed in terms of the difference of sensing the interfacial coupling in the two cases due to atomic steps. PACS classification codes 75-60; 75-70; 81-15G Keywords: Exchange coupling; Anisotropy - uniaxial; Anisotropy - unidirectional; Thin films *Corresponding author. Tel.: +33 5 61 55 61 85; e-mail: mamy@insa-tlse.fr.