Europhys. Lett. 19 (8) pp 711-716 (1992) Antiferromagnetci Coupling of a Cr Overlayer to Fe(100) F. U. Hillebrecht, Ch. Roth, R. Jungblut, E. Kisker and A> Bringer The magnetic moment of Cr overlayers deposited on Fe(100) was investigated by spin-resolved core level photoemission. data for the Cr 3p level show that a monolayer of Cr is ferromagnetically ordered with a magnetic moment oriented antiparallel to the Fe moments. The results suggest that at room temperature the moment of a Cr monolayer on Fe is of the order of 0.5 to 1 mu_Bohr per Cr atom